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Environmental radiological monitoring and risk assessment in shale gas areas

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机构: [1]Affiliated Cancer Hospital, School of Medicine, University of Electronic Science and Technology of China, Chengdu, 611731, PR China [2]College of Nuclear Technology and Automation Engineering, Chengdu University of Technology, Chengdu, 610059, Sichuan, PR China [3]Applied Nuclear Technology in Geosciences Key Laboratory of Sichuan Province, Chengdu University of Technology, Chengdu, 610059, PR China [4]Chongqing Radiation Environment Supervision and Management Station, Chongqing, 401123, PR China [5]SCMPA Key Laboratory for Quality Research and Control of Chemical Medicine, Chengdu Institute for Drug Control, Chengdu, 610000, PR China
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关键词: Naturally occurring radioactive materials (NORM) Shale gas extraction Environmental radiation exposure Radionuclide migration Radioactive wastewater treatment

摘要:
Naturally occurring radioactive materials (NORM) are present in waste generated during shale gas drilling activities and pose potential risks to the environment, drawing increasing public and scientific attention. In this study, soil, wastewater and effluent samples were collected across multiple operational stages of shale gas development in Southwest China. A combination of in-situ gamma absorbed dose rate in air, soil radon concentration, radionuclide activity concentrations, and conventional hazard indices was used to evaluate environmental radioactivity and potential occupational exposure. The results showed that both the gamma absorbed dose rates and soil radioactivity were comparable to those observed in other oil and gas fields, that were strongly correlated with uranium-series nuclides. A strong linear relationship between 238U and 226Ra, indicating the two radionuclides were in near radioactive equilibrium within the soil. The 210Pb/226Ra ratio was consistently greater than 1 and increased with platform operation time, suggesting an accumulation of radon progeny. Discrepancies between measured and calculated dose rates highlighted the need to prioritize direct measurements in dose assessments. Worker dose assessments revealed annual effective doses below 1 mSvy-1. Furthermore, elevated concentrations of 226Ra, 228Ra, and 40K were detected in untreated-water, which could be effectively reduced by existing treatment technologies. These findings provide a baseline for radiological risk evaluation in shale gas fields and highlight the necessity for continuous monitoring and wastewater management.Copyright © 2025 Elsevier Inc. All rights reserved.

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出版当年[2025]版:
大类 | 2 区 环境科学与生态学
小类 | 2 区 环境科学 2 区 公共卫生、环境卫生与职业卫生
最新[2025]版:
大类 | 2 区 环境科学与生态学
小类 | 2 区 环境科学 2 区 公共卫生、环境卫生与职业卫生
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出版当年[2024]版:
Q1 ENVIRONMENTAL SCIENCES Q1 PUBLIC, ENVIRONMENTAL & OCCUPATIONAL HEALTH
最新[2024]版:
Q1 ENVIRONMENTAL SCIENCES Q1 PUBLIC, ENVIRONMENTAL & OCCUPATIONAL HEALTH

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第一作者机构: [1]Affiliated Cancer Hospital, School of Medicine, University of Electronic Science and Technology of China, Chengdu, 611731, PR China [2]College of Nuclear Technology and Automation Engineering, Chengdu University of Technology, Chengdu, 610059, Sichuan, PR China [3]Applied Nuclear Technology in Geosciences Key Laboratory of Sichuan Province, Chengdu University of Technology, Chengdu, 610059, PR China
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